Celtic Predator looked the coolest, but he died pretty easily. Gonna have to jump on the bandwagon though and go with the original Jungle Hunter. Wristblades and and Plasma Caster like a bamf.
I also really liked the main predator from Predator: Concrete Jungle (the game)

I liked the idea behind Falconer in Predators, especially being the Pred drone aeriel scout.... The mask was fresh and original. He was a scout. Lightly armoured, fast with a deadly looking single blade.

Wolf a close second. There was a personality to him, something a lot of the other predators lacked.

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