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There is no direct way to do this yet in Spiceworks. You could do something like the following though, and it might be enough to get you by:

Go to Settings->Advanced and add a custom attributed called something like "For Service". You could make this a choice list with your current list of IT Services. Save this, and then go to the General view of each Asset that you want to assign to a Service. You can then select edit and assign the asset to a service.

Now/later, go to the top inventory view, select the View browse (right side of the top bar), then select All Computers "For Service" and you will have your lists of assets by service. It should also be possible to write a custom report that lists these all out as well.