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Professor Jolliff's teaaching and research focus is on the Moon and Mars, the materials that make up their surfaces and interiors, and what they tell about the planet's history.

Jolliff is a member of the Mars Exploration Rovers operations team and the Lunar Reconnaissance Orbiter Camera science team. He was the principal investigator of the "MoonRise" New Frontiers mission proposal, which competed though a Phase A concept study as one of three finalists for NASA's medium-class planetary exploration mission program.