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I'd have to say it's a tie for me between Pan/Simisage, Joltik/Galvantula, and Chandelure. I really just don't know, they're all great, and in the case of the latter two, have really interesting typings~

I like Petilil/Lilligant and Whimsicott since the Grass type is one of my favourite types and these new Grass additions are both good Pokémon and I've also used them both in my active teams, Lilligant in Black and Whimsicott in Black 2. I also like Snivy but I never chose it as my starter. I have it though.

Psychic type is also a type I like and Munna/Musharna were one of my favs in this Gen as well. Especially Munna, it is so cute! ♥ Other Pokémon I like are Krookodile (just awesome badass-croc Pokémon!), Hydreigon (cool and feral Dragon type), Deerling (very cute and I like how it changes its colours) and Chandelure (very noice idea and design).

Personally, most of the 5th Gen Pokémon were disappointment to me and I don't think they were very original. Though there is Pokémon I like but most of them I didn't like at all. But I liked the thing that in B/W you didn't have any of the old Pokémon in Unova before beating the league so you had to pick your team among the new Pokémon. I just hope that I like the 6th gen Pokémon more and that there is more designs and Pokémon I like than in 5th Gen.

I love Litwick - i love its emo look about it. Im kinda glad Game Freak made a part ghost type that was less.... Creepy (although lampents pokedex is totes disturbing) Plus, Chandelures just pure awesomeness.
I also like Gigalith for its coolness, but Litwick/Chandelure just beats it by a landslide.

My favorite fifth Gen Pokemon is easily Scrafty. He's just awesome! With the unique typing of Dark/Fighting it's just interesting to see a Pokemon comprised of two complete type opposites. Besides, who doesn't like a Pokemon that has a hoodie.
Well, I wish it were a hoodie anyway, but just the hood is good enough for me.

Out of the small 20 pokémon I like from Gen 5, Bravialry, Volcarona, Reshiram and Zekrom are my favourite. It's got a fantastic design that really outshines almost all other Flying-type pokémon. Volcarona is a great design execution and a great pokémon as a whole. Reshiram and Zekrom may be mascots for the worst Pokémon games in the main series, but I can deny they are well-designed pokémon.