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Rare Candies aren't a good training method, because you don't earn the EVs that come about from actually battling. A level 100 juiced on Rare Candies is significantly weaker than one that was raised normally.
I would suggest a Lucky Egg + the Stadiums + Royal Unova + Cheren and Bianca + Audinos Black City (if applicable). If you go at a fair pace, I would say you could get a level 1 to level 100 in about a week.

But you can EV Train Pokémon that are actually Lv 100. So you can EV train after you Level Up your 'mons.

Simple. Lucky Egg or Exp. Share, Audino's, trading over pokemon, strong wild pokemon (Giant Chasm is a good place, as well as Abundant Shrine and Challenger's Cave), and strong trainers like Morimoto, Bianca, Cheren, the Nimbasa sports althetes and of course the Elite Four. Keep on grinding.

Okay. I can get 3 Pokémon to Lv. 100 in one day using this method. It is important to note you will need 2 DSes and 2 BW games and a fully levelled up Entree on the game you're training your Pokémon on. We'll call that game #1. Game #2 is there to simply give the MAX Power to game #1. Got it? Okay. Here's what you do.

Have game #2 give the Exp. Point Power MAX to game #1. (It lasts a whole hour and gives ×2 Exp rate) Go to the first part of Route 14, just north of Black City/White Forest. Ride your bike left and right until Audinos appear.
You can increase the effectiveness of the Exp. gain by giving the Pokémon a Lucky Egg, and even more so if it was traded to you.
Furthermore, try to have 5 Lv. 100 Pickup ability Pokémon in your party as well. They'll be useful in obtaining PP Ups and Rare Candies.

It would be advisable to EV train any Pokémon you plan on training - before you start Audino hunting, because Audinos give 2HP EVs for each one you slay.

This is a round about method but getting ''pick-up'' ability pokemon into the levels rare candy becomes a 10% chance and a 10% chance after each fight to pick up an item. I usually habe my lv100 boosting with exp share, Pokemon i'm EV training, HM Slave (Box it if possible) and x3-4 pickup pokemon.

Assuming you maxed at least to abilitys with vitamins and are battling 2 point EV givers thats 310 battles... Only 9-12 rare candies per maxed EV pokemon on average but being able to skip 88-100 saves quite alot of time. Then you have all the battling to level 90+ should give at least 10 rare candies if traded through wild pokemon not to mention an abundant of other goodies.

Do use a Lucky egg, the most important item next to Exp share.

Or... if your lucky enough to have a friend or own two DS's trade the pokemon over for the x1.7 modifer in the other game.

Once your Pokemon are strong enough, just keep battling all of the powerful trainers in Unova. This includes the Elite Four, Cynthia (Spring after beating her the first time) and Miyamoto (Gamefreak HQ). They are all at pretty high levels, so try that

Talk to Cheren at Route 5 an then battle him right outside the league in the cave entrance to the right. You can battle him once a day.

There's a house where you can fight two rotation battles if you play Pokemon Black or two triple battles if you play Pokemon White once per day.

I Friday nights you can battle a biker on Tubeline Bridge.

In Undella you can battle the Riches once a day. First one, then the next day two, and so on until the sixth member appears. In order to keep getting to battle them once a day, make sure to lose to the sixth member. Don't worry about losing money, you get at least 12,000 for each battle and each battle increases the amount.

You can battle Cynthia once a day at her home in Undella during Spring.

If you have Pokemon Black, Black City might have trainers for you to battle.

Both stadiums have a bunch of trainers you can battle daily at Nimbasa as well a a little battle once a day at the ferris wheel.

In Castelia at the GAMEFREAK building on the 22nd floor, fight Morimoto once a day.

The Royal Unova can be battled once a day.

You can also battle Bianca on Saturday and Sunday at the lab after beating the League a second time.

These are the dailies I do to level up. I also equip a lucky egg to all pokemon I'm leveling and if possible get the boost from being a traded pokemon. Also, I save before entering either of the stadiums. This way, I can keep trying to battle trainers I want to battle. I always make sure to battle the doctor once a day so I get a max revive from beating him plus a LOT of exp from his audino which is great for any level to fight since it, as far as I've seen, doesn't deal damage. But if you want to keep restarting for certain trainers, just know that once you save after entering either stadium, the other stadium you haven't, you can't keep reseting to get certain trainers in there as well.

C-Gear Powers (Exp Power +++) Yes, it's really good - I used to up 20+ Lv in only 1 battle.

Speaking of that...there is a trainer in one of the stadiums with a Lv65 Audino...I wonder how much EXP a Lv1 Pokemon from another country, holding the Lucky Egg and with Exp Power +++ activated would get? Would definitely be great to test it out... Especially ones in the Erratic group...

Speaking of that...there is a trainer in one of the stadiums with a Lv65 Audino...I wonder how much EXP a Lv1 Pokemon from another country, holding the Lucky Egg and with Exp Power +++ activated would get? Would definitely be great to test it out... Especially ones in the Erratic group...

Well my pokemon I got from a trade that was from level 73-80 something holding the lucky egg got exp with five digits.