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Memory 1 - The Hidden City

Since all of the guards in the entire area will not be suspicious of Ezio, he can roam around the entire area as long as he doesn't cause any trouble. Stick with the main objective and you should get 100% Sync easily.

Once you reach Cappadocia, make your way up the giant stairway and enter the mountain entrance towards the inner mountain. After a short cutscene, enter the city and hop along the shanties towards the giant mountain spiral in the middle of Cappodocia.

Climb up to the very top and activate the Viewpoint to fill in the GPS. Use a Leap of Faith to the bottom and then make your way towards the green area. Activate Eagle Sense and walk around spying on groups of people until you locate the target.

After the target is confirmed, confront the spy and they will make a dash for it. Quickly chase the spy through the alleys until you finally corner them near a doorway to complete the mission.