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Id say pretty much anything done by Key, which would be Air, Kanon, Clannad, and such. I also really like the art direction in Soul Eater, although its not the prettiest ive ever seen, its just different from anything else that ive seen

O.K as an older fan let me put forward Ah! My Goddess the original OVA. Remember there was no fancy CGI when this was made and it still looks good today. Also Akira. Again an old Anime that still looks absolutely superb.

All that are done by Watase Yuu are my favorite. I love how she illustrates the characters to tell the story in many different views. If you look closer to her artworks, you'll notice a story behind each of her artworks.