She has a nice body, i love her psychotic tendencies, and her taunts...even some of her moves are kind of....moving on
mad moxxi from borderlands, the psychotic-ness of juri, though i will admit i don't really like the way she looks that much, but she's so much fun that it makes up for it

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heather mason from silent hill 3
she's cute, snarky, and probably my favorite protagonist from these games. did i mention that she's also really cool?

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(though it's a very loose definiton of a video game) hanako from katawa shoujo
She's pretty, cute, nice (unless you get the bad ending...which i havent yet ) and (imo) her route is the best, which gives her extra points.

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My last one for girls...umm...hmm...Tabby from .hack//GU 3? nah. erm...OH
Reika Kuze from fatal frame 3

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She's pretty, i like her tattoos, and she's also probably my favorite character in the games. speaking of which, i need to finish them!

now for guys
Dante (how can this guy NOT make the list?) from DMC

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a tie between ryu from street fighter, i really don't know why but i just think he's cute

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and vega from street fighter, he's pretty, has a nice body, wonderfully psychotic. and you have to admit, the mask + claws is sexy

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Gabriel belmont, i havent even played a castlevania game since symphony of the night, but gabriel looks kinda like level 0 alucard, plus he's a belmont, so he probably has an affinity for whips

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another tie
Pyramid head/james sunderland/Alex shepherd
Pyramid head

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...knowing me, is anyone really surprised? actually, even if you don't know me, just look at my other choices. He has a nice body, if the hints are anything to go by, he probably looks like james under the mask, speaking of which...
james

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again, if the hints are true and pyramid head looks like james, then james probably also has a nice body. The difference between the two is obvious though, james in nice and sweet (well for most of the game anyway) and his social awkwardness is just adorable
and alex