We revisit and supplement the description of gravity waves based on perturbation expansions in Lagrangian coordinates. A general analytical framework is developed to derive a second-order Lagrangian solution to the motion of arbitrary surface gravity wave fields in a compact and vectorial form. The result is shown to be consistent with the classical second-order Eulerian expansion by Longuet-Higgins (J. Fluid Mech., vol. 17, 1963, pp. 459-480) and is used to improve the original derivation by Pierson (1961 Models of random seas based on the Lagrangian equations of motion. Tech. Rep. New York University) for long-crested waves. As demonstrated, the Lagrangian perturbation expansion captures nonlinearities to a higher degree than does the corresponding Eulerian expansion of the same order. At the second order, it can account for complex nonlinear phenomena such as wave-front deformation that we can relate to the initial stage of horseshoe-pattern formation and the Benjamin-Feir modulational instability to shed new light on the origins of these mechanisms.