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Sharing a bit about their wedding, Jolie recalls to VF contributing editor Janine di Giovanni the vows that her children wrote for her and Pitt. "They did not expect us never to fight, but they made us promise to always say, 'Sorry,' if we do," she explains. "So they said, 'Do you?,' and we said, 'We do!'"

Now that they're married, Pitt and Jolie are gearing up to the return to the big screen together, a first since their 2005 film, "Mr. and Mrs. Smith." Jolie directs and stars alongside Pitt in "By the Sea," and she confesses jokingly, "A few friends asked if we were crazy. [A film about] a married couple going through some difficulties ...and I'm directing him."

When Jolie isn't caring for her family or being a major movie star, she's working on making the world a better place. But given all her charitable efforts around the globe, would she ever consider running for a political office? "I am open," Jolie admits.