Before Steve Buscemiwas a household name, he was known everywhere as “Oh, That Guy!” With his unforgettable face a neurotic delivery that lends itself to crime movies and comedies alike (imagine a Christopher Walken/Don Knotts love child), Buscemi is a fixture in Coen Brothers films, which typically fit both genres. His most beloved roles have been in those and other indie movies, such as Ghost World and Reservoir Dogs, but he’s also been an inimitable TV presence in The Sopranos, 30 Rock and Boardwalk Empire, and he voiced one of the most delicious cartoon villains ever—the lizard-like Randall of Monsters, Inc. He’s the voice of a new villain in The Boss Baby, opening March 30.