I am looking for some good and interesting music. Music along the lines of MC Lars, Atom and His Package, and MC Chris. Music that normally can't be put into a definitive category, but blend the genres. Anyone have any suggestions?

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I'm not familiar with the stuff you've mentioned, but here's something that blends multiple genres seamlessly.

The band is Ozomatli and the album is Street Signs. It's a seamless blend of Latin music, Middle Eastern music, and hip-hop.

If you're more into a fusion of funk, rock, jazz, blues, and hip-hop, definitely check out Screaming Headless Torsos. Their album called 1995 is awesome.

One group that I've been getting into recently is called Ivory Tower (http://www.ivorytowermusic.com). Their On a Far and Distant Shore is quite refreshing to listen to- it has a new age, poppy sound. I like it.

If you like your genre blending to have a familiar feel, definitely check out Antigone Rising. This all female band encompass elements of rock, folk, blues, country, pop...